Normal state specific heat in the cuprate superconductors La2xSrxCuO4 and Bi2+ySr2xyLaxCuO6+δ near the critical point of the pseudogap phase

C. Girod, D. LeBoeuf, A. Demuer, G. Seyfarth, S. Imajo, K. Kindo, Y. Kohama, M. Lizaire, A. Legros, A. Gourgout, H. Takagi, T. Kurosawa, M. Oda, N. Momono, J. Chang, S. Ono, G.-q. Zheng, C. Marcenat, L. Taillefer, and T. Klein
Phys. Rev. B 103, 214506 – Published 7 June 2021
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Abstract

The specific heat C of the cuprate superconductors La2xSrxCuO4 and Bi2+ySr2xyLaxCuO6+δ was measured at low temperatures (down to 0.5 K) for dopings p close to p, the critical doping for the onset of the pseudogap phase. A magnetic field up to 35 T was applied to suppress superconductivity, giving direct access to the normal state at low temperatures, and enabling a determination of Ce, the electronic contribution to the normal-state specific heat at T0. In La2xSrxCuO4 at x=p=0.22, 0.24 and 0.25, Ce/T=15to16mJmol1K2 at T=2K, values that are twice as large as those measured at higher doping (p>0.3) and lower doping (p<0.15). This confirms the presence of a broad peak in the doping dependence of Ce at p0.19 as previously reported for samples in which superconductivity was destroyed by Zn impurities. Moreover, at those three dopings, we find a logarithmic growth as T0 such that Ce/TBln(T0/T). The peak versus p and the logarithmic dependence versus T are the two typical thermodynamic signatures of quantum criticality. In the very different cuprate Bi2+ySr2xyLaxCuO6+δ, we again find that Ce/TBln(T0/T) at pp, strong evidence that this ln(1/T) dependence of the electronic specific heat—first discovered in the cuprates La1.8xEu0.2SrxCuO4 and La1.6xNd0.4SrxCuO4—is a universal property of the pseudogap critical point.

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  • Received 20 January 2021
  • Revised 14 May 2021
  • Accepted 14 May 2021

DOI:https://doi.org/10.1103/PhysRevB.103.214506

©2021 American Physical Society

Physics Subject Headings (PhySH)

  1. Physical Systems
Condensed Matter, Materials & Applied Physics

Authors & Affiliations

C. Girod1,2, D. LeBoeuf3, A. Demuer3, G. Seyfarth3, S. Imajo4, K. Kindo4, Y. Kohama4, M. Lizaire2, A. Legros2, A. Gourgout2, H. Takagi5, T. Kurosawa6, M. Oda6, N. Momono7, J. Chang8, S. Ono9, G.-q. Zheng10,11, C. Marcenat12,*, L. Taillefer2,13,†, and T. Klein1,‡

  • 1Institut Néel, Université Grenoble Alpes, CNRS, Grenoble INP, F-38000 Grenoble, France
  • 2Département de Physique, and RQMP, Institut Quantique, Université de Sherbrooke, Sherbrooke, Québec J1K 2R1, Canada
  • 3Université Grenoble Alpes, INSA Toulouse, Université Toulouse Paul Sabatier, EMFL, CNRS, LNCMI, F-38000 Grenoble, France
  • 4Institute for Solid State Physics, University of Tokyo, Kashiwa, Chiba 277-8581, Japan
  • 5Department of Advanced Materials, University of Tokyo, Kashiwa 277-8561, Japan
  • 6Department of Physics, Hokkaido University, Sapporo 060-0810, Japan
  • 7Muroran Institute of Technology, Muroran 050-8585, Japan
  • 8Physik-Institut, Universitat Zurich, Winterthurerstrasse 190, CH-8057 Zurich, Switzerland
  • 9Central Research Institute of Electric Power Industry, Materials Science Research Laboratory, 2-6-1 Nagasaka, Yokosuka, Kanagawa, Japan
  • 10Department of Physics, Okayama University, Okayama 700-8530, Japan
  • 11Institute of Physics, Chinese Academy of Sciences, Beijing National Laboratory for Condensed Matter Physics, Beijing 100190, China
  • 12Université Grenoble Alpes, CEA, Grenoble INP, IRIG, PHELIQS, 38000 Grenoble, France
  • 13Canadian Institute for Advanced Research, Toronto, Ontario M5G 1M1, Canada

  • *christophe.marcenat@cea.fr
  • louis.taillefer@usherbrooke.ca
  • thierry.klein@neel.cnrs.fr

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Issue

Vol. 103, Iss. 21 — 1 June 2021

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