Magnetic ordering and spin-liquid state of YMnO3

Junghwan Park, J.-G. Park, Gun Sang Jeon, Han-Yong Choi, Changhee Lee, W. Jo, R. Bewley, K. A. McEwen, and T. G. Perring
Phys. Rev. B 68, 104426 – Published 23 September 2003
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Abstract

We have measured the bulk properties as well as the elastic and inelastic neutron scattering of YMnO3 in order to understand the static and dynamic properties of the Mn moments. Our measurements clearly show that above TN there are short range correlations between spins at the nearest neighbor and next nearest neighbor Mn sites, which also fluctuate in time. This, together with other bulk properties, demonstrates the presence of a spin liquid phase above TN arising from the geometrically frustrated Mn moments. Below TN, a well-defined spin wave develops and we can understand the experimentally measured spin wave spectrum in terms of a Heisenberg Hamiltonian with a small easy plane anisotropy. However, even in the ordered phase we have found evidence of short range spin correlations.

  • Received 28 June 2002

DOI:https://doi.org/10.1103/PhysRevB.68.104426

©2003 American Physical Society

Authors & Affiliations

Junghwan Park1, J.-G. Park2,3,*, Gun Sang Jeon2, Han-Yong Choi2, Changhee Lee4, W. Jo5, R. Bewley6, K. A. McEwen7, and T. G. Perring6

  • 1Department of Physics, Inha University, Incheon 402-751, Korea
  • 2Department of Physics and Institute of Basic Science, SungKyunKwan University, Suwon 440-746, Korea
  • 3Center for Strongly Correlated Materials Research, Seoul National University, Seoul 151- 742, Korea
  • 4Neutron Physics Laboratory, Korea Atomic Energy Research Institute, Daejon 305-600, Korea
  • 5Geballe Laboratory for Advanced Materials, Stanford University, California 94305, USA
  • 6ISIS Facility, Rutherford Appleton Laboratory, Chilton, Didcot OX11 0QX, United Kingdom
  • 7Department of Physics and Astronomy, University College London, Gower Street, London WC1E 6BT, United Kingdom

  • *Author to whom correspondence should be addressed. Email address: jgpark@skku.ac.kr

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Vol. 68, Iss. 10 — 1 September 2003

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