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Exciton valley dynamics probed by Kerr rotation in WSe2 monolayers

C. R. Zhu, K. Zhang, M. Glazov, B. Urbaszek, T. Amand, Z. W. Ji, B. L. Liu, and X. Marie
Phys. Rev. B 90, 161302(R) – Published 6 October 2014

Abstract

We have experimentally studied the pump-probe Kerr rotation dynamics in WSe2 monolayers. This yields a direct measurement of the exciton valley depolarization time τv. At T=4K, we find τv6 ps, a fast relaxation time resulting from the strong electron-hole Coulomb exchange interaction in bright excitons. The exciton valley depolarization time decreases significantly when the lattice temperature increases, with τv being as short as 1.5 ps at 125 K. The temperature dependence is well explained by the developed theory, taking into account the exchange interaction and fast exciton scattering time on the short-range potential.

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  • Received 21 July 2014
  • Revised 10 September 2014

DOI:https://doi.org/10.1103/PhysRevB.90.161302

©2014 American Physical Society

Authors & Affiliations

C. R. Zhu1, K. Zhang1,2, M. Glazov3, B. Urbaszek4, T. Amand4, Z. W. Ji2, B. L. Liu1,*, and X. Marie4,†

  • 1Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, P.O. Box 603, Beijing 100190, People's Republic of China
  • 2School of Physics, Shandong University, Jinan 250100, China
  • 3Ioffe Physical-Technical Institute of the RAS, 194021 St. Petersburg, Russia
  • 4Université de Toulouse, INSA-CNRS-UPS, LPCNO, 135 Avenue de Rangueil, 31077 Toulouse, France

  • *blliu@aphy.iphy.ac.cn
  • marie@insa-toulouse.fr

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Issue

Vol. 90, Iss. 16 — 15 October 2014

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