Computational studies of history dependence in nematic liquid crystals in random environments

Amid Ranjkesh, Milan Ambrožič, Samo Kralj, and Timothy J. Sluckin
Phys. Rev. E 89, 022504 – Published 13 February 2014

Abstract

Glassy liquid crystalline systems are expected to show significant history-dependent effects. Two model glassy systems are the RAN and SSS (sprinkled silica spin) lattice models. The RAN model is a Lebwohl-Lasher lattice model with locally coupled nematic spins, together with uncorrelated random anisotropy fields at each site, while the SSS model has a finite concentration of impurity spins frozen in random directions. Here Brownian simulation is used to study the effect of different sample histories in the low temperature regime in a three-dimensional (d=3) model intermediate between SSS and RAN, in which a finite concentration p<pc (pc the percolation threshold) of frozen spins interacts with neighboring nematic spins with coupling W. Simulations were performed at temperature TTNI/2 (TNI the bulk nematic-isotropic transition temperature) for temperature-quenched and field-quenched histories (TQH and FQH, respectively), as well as for temperature-annealed histories (AH). The first two of these limits represent extreme histories encountered in typical experimental studies. Using long-time averages for equilibrated systems, we calculate orientational order parameters and two-point correlation functions. Finite-size scaling was used to determine the range of the orientational ordering, as a function of coupling strength W,p and sample history. Sample history plays a significant role; for given concentration p, as disorder strength W is increased, TQH systems sustain quasi-long-range order (QLRO) and short-range order (SRO). The data are also consistent with a long-range order (LRO) phase at very low disorder strength. By contrast, for FQH and p0.1, only LRO and QLRO occur within the range of parameters investigated. The crossover between regimes depends on history, but in general, the FQH phase is more ordered than the AH phase, which is more ordered than the TQH phase. However, at temperatures close to the isotropic-nematic phase transition of pure samples we observe SRO for p=0.1 even for FQH. We detect also in the QLRO phase a domain-type structural pattern, consistent with ideas introduced by Giamarchi and Doussal [Phys. Rev. B 52, 1242 (1995)] on superconducting flux lattices. In the weak-disorder limit the orientational correlation length obeys the Larkin-Imry-Ma scaling ξD2/(4d).

    • Received 23 October 2013

    DOI:https://doi.org/10.1103/PhysRevE.89.022504

    ©2014 American Physical Society

    Authors & Affiliations

    Amid Ranjkesh1,*, Milan Ambrožič1,†, Samo Kralj1,2,‡, and Timothy J. Sluckin3,§

    • 1Faculty of Natural Sciences and Mathematics, University of Maribor, Koroška 160, 2000 Maribor, Slovenia
    • 2Condensed Matter Physics Department, Jožef Stefan Institute, Jamova 39, 1000 Ljubljana, Slovenia
    • 3Division of Mathematical Sciences, University of Southampton, Southampton, SO17 1BJ, United Kingdom

    • *amid.ranjkesh@uni-mb.si
    • milan.ambrozic@uni-mb.si
    • samo.kralj@uni-mb.si
    • §T.J.Sluckin@soton.ac.uk

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    Issue

    Vol. 89, Iss. 2 — February 2014

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